Mode-multiplexing deep-strong light-matter coupling

dc.contributor.authorMornhinweg, Joshua
dc.contributor.authorDiebel, Laura Katharina
dc.contributor.authorHalbhuber, Maike
dc.contributor.authorPrager, Michael
dc.contributor.authorRiepl, Josef
dc.contributor.authorInzenhofer, Tobias
dc.contributor.authorBougeard, Dominique
dc.contributor.authorHuber, Rupert
dc.contributor.authorLange, Christoph
dc.date.accessioned2024-08-09T13:16:11Z
dc.date.available2024-08-09T13:16:11Z
dc.date.issued2024-02-28
dc.description.abstractDressing electronic quantumstates with virtual photons creates exotic effects ranging from vacuum-field modified transport to polaritonic chemistry, and squeezing or entanglement of modes. The established paradigm of cavity quantum electrodynamics maximizes the light-matter coupling strength ΩR=ωc, defined as the ratio of the vacuumRabi frequency and the frequency of light, by resonant interactions. Yet, the finite oscillator strength of a single electronic excitation sets a natural limit to ΩR=ωc. Here, we enter a regime of record-strong light-matter interaction which exploits the cooperative dipole moments of multiple, highly non-resonant magnetoplasmon modes tailored by ourmetasurface. This creates an ultrabroadband spectrum of 20 polaritons spanning 6 optical octaves, calculated vacuum ground state populations exceeding 1 virtual excitation quantum, and coupling strengths equivalent to ΩR=ωc =3:19. The extreme interaction drives strongly subcycle energy exchange between multiple bosonic vacuum modes akin to high-order nonlinearities, and entangles previously orthogonal electronic excitations solely via vacuum fluctuations.en
dc.identifier.urihttp://hdl.handle.net/2003/42642
dc.identifier.urihttp://dx.doi.org/10.17877/DE290R-24479
dc.language.isoenen
dc.relation.ispartofseriesNature communications;15
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/en
dc.subject.ddc530
dc.titleMode-multiplexing deep-strong light-matter couplingen
dc.typeTexten
dc.type.publicationtypeArticleen
dcterms.accessRightsopen access
eldorado.secondarypublicationtrue
eldorado.secondarypublication.primarycitationMornhinweg, Joshua, Laura Katharina Diebel, Maike Halbhuber, Michael Prager, Josef Riepl, Tobias Inzenhofer, Dominique Bougeard, Rupert Huber, und Christoph Lange. „Mode-Multiplexing Deep-Strong Light-Matter Coupling“. Nature Communications 15 (2024). https://doi.org/10.1038/s41467-024-46038-9en
eldorado.secondarypublication.primaryidentifierhttps://doi.org/10.1038/s41467-024-46038-9

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