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dc.contributor.authorKeuchel, Florian-
dc.contributor.authorHeinlein, Moritz-
dc.contributor.authorHohlmann, Jan-
dc.contributor.authorAgar, David W.-
dc.date.accessioned2024-03-04T12:22:06Z-
dc.date.available2024-03-04T12:22:06Z-
dc.date.issued2022-03-10-
dc.identifier.urihttp://hdl.handle.net/2003/42370-
dc.identifier.urihttp://dx.doi.org/10.17877/DE290R-24207-
dc.description.abstractSo far, no complete reaction mechanism has been proposed for high temperature chlorination and pyrolysis of methane. Various mechanisms for the description of this reaction pathway are combined and compared in this paper. This adaptation shows that the gas phase pyrolysis of methane and methyl chloride can be combined with surface reactions via nucleation from the gas phase or on the reactor wall to reproduce the product spectrum. In addition, kinetic parameters for a global simplified one-step mechanism focused on the formation of carbon are fitted to available experimental data.en
dc.language.isoende
dc.relation.ispartofseriesChemie - Ingenieur - Technik;94(5)-
dc.rights.urihttps://creativecommons.org/licenses/by-nc/4.0/de
dc.subjectChlorinationen
dc.subjectHigh temperatureen
dc.subjectKinetic mechanismen
dc.subjectMethane pyrolysisen
dc.subjectSimulationen
dc.subject.ddc660-
dc.titleAnalysis and simplification of kinetic models for methane chlorination and pyrolysisen
dc.typeTextde
dc.type.publicationtypeResearchArticlede
dc.subject.rswkChlorierungsreaktionde
dc.subject.rswkHochtemperaturchemiede
dc.subject.rswkReaktionskinetikde
dc.subject.rswkMethande
dc.subject.rswkPyrolysede
dc.subject.rswkSimulationde
dcterms.accessRightsopen access-
eldorado.secondarypublicationtruede
eldorado.secondarypublication.primaryidentifierhttps://doi.org/10.1002/cite.202100179de
eldorado.secondarypublication.primarycitationKeuchel, F., Heinlein, M., Hohlmann, J. and Agar, D.W. (2022), Analysis and Simplification of Kinetic Models for Methane Chlorination and Pyrolysis. Chemie Ingenieur Technik, 94: 712-719. https://doi.org/10.1002/cite.202100179en
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