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Signature of ergodicity in the dynamic response of amorphous systems

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Date

1992

Authors

Böhmer, Roland
Chamberlin, R. V.
Sanchez, E.
Angell, C. A.

Journal Title

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Publisher

The American Physical Society

Abstract

We have analyzed dynamical measurements from materials near their liquid-glass transition. The primary response is accurately characterized by a model for dispersive excitations on specific distributions of independently relaxing domains. Liquids have an equilibrium (Gaussian) distribution of domain sizes, which changes abruptly to a locally random (Poisson-like) distribution in the glass. When quenched to a temperature initially in the glass phase, after a definite anneal time, the Poisson-like distribution changes abruptly back to the Gaussian distribution characteristic of a liquid.

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Citation

Chamberlin, R. V.; Böhmer, R.; Sanchez, E.; Angell, C. A.: Signature of ergodicity in the dynamic response of amorphous systems. In: Physical Review B Nr. 9, Jg. 46(1992), S. 5787-5790, doi: 10.1103/PhysRevB.46.5787 .