Authors: | Böhmer, Roland Chamberlin, R. V. Diezemann, G. Geil, B. Heuer, A. Hinze, G. Kuebler, S. C. Richert, R. Schiener, B. Sillescu, H. Spiess, H. W. Tracht, U. Wilhelm, M. |
Title: | Nature of the non-exponential primary relaxation in structural glass-formers probed by dynamically selective experiments |
Language (ISO): | en |
Abstract: | Several experimental methods feature the potential to distinguish between slow and fast contributions to the non-exponential, ensemble averaged primary response in glass-forming materials. Some of these techniques are based on the selection of subensembles using multi-dimensional nuclear magnetic resonance, optical bleaching, and non-resonant spectral hole burning. Others, such as the time-dependent solvation spectroscopy, measure microscopic responses induced by local perturbations. Using several of these methods it could be demonstrated for various glass-forming materials that the non-exponential relaxation results from a superposition of dynamically distinguishable entities. The experimental observation that subensembles can be selected efficiently indicates a large degree of heterogeneity. The intrinsic response is compatible with single exponential relaxation. |
URI: | http://hdl.handle.net/2003/25474 http://dx.doi.org/10.17877/DE290R-3300 |
Issue Date: | 1999-04-08 |
Provenance: | Elsevier |
URL: | http://dx.doi.org/10.1016/S0022-3093(98)00581-X |
Citation: | Böhmer, R.; Chamberlin, R. V.; Diezemann, G.; Geil, B.; Heuer, A.; Hinze, G.; Kuebler, S. C.; Richert, R.; Schiener, B.; Sillescu, H.; Spiess, H. W.; Tracht, U.; Wilhelm, M.: Nature of the non-exponential primary relaxation in structural glass-formers probed by dynamically selective experiments. In: Journal of Non-Crystalline Solids Jg. 235-237(1998), S. 1-9, doi: 10.1016/S0022-3093(98)00581-X. |
Appears in Collections: | Böhmer, Roland Prof. Dr. |
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