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Nitrogen-vacancy (NV) centers in diamond have become an important tool for quantumtechnologies. All of these applications rely on long coherence times of electron and nuclear spinsassociated with these centers. Here, we study the energy level anti-crossings of an NV center indiamond coupled to a first-shell13C nuclear spin in a small static magnetic field. These levelanti-crossings (LACs) occur for specific orientations of the static magnetic field due to the strongnon-secular components of t...
Excitons are fundamental electronic excitations in a semiconductor. They are bound states consisting of an electron in the conduction band and a positively charged hole in the valence band. They have hydrogen-like properties and are therefore referred to as the hydrogen analogues in solid states. In the semiconductor Cuprous Oxide, Cu2O, highly excited states of excitons can be observed with principal quantum numbers up to n = 25. These states are called Rydberg excitons in analogy to th...
In this thesis, two searches for the pair production of vector-like top (VLT) and vector-like bottom (VLB) quarks are presented using 36.1 fb⁻¹ and 139 fb⁻¹ of data. The data was taken at √s = 13 TeV in proton-proton collisions with the ATLAS detector, which is one of the major experiments at the Large Hadron Collider at CERN. The decay signature of this search for TT and BB production is characterized by the presence of a Z-boson, which is reconstructed from two opposite-charge same-flavor l...
It is important to exploit particle detectors for the detection and identification of electrons and photons in the best possible way, as it is adressed in this thesis by discussing three different application examples of precisely measuring electrons and photons at high-energy physics and test beam experiments. Firstly, the optimization of the photon identification within the ATLAS detector at the LHC is investigated. Appropriate selection criteria are needed to efficiently discriminate pr...
In magnetic semiconductors the optical spectrum and, in particular, the absorption edge representing the band-gap are strongly affected by the onset of the magnetic order. This contribution to the band-gap energy has hitherto been described theoretically in terms of a Heisenberg Hamiltonian, in which a delocalized conduction carrier is coupled to the localized magnetic moments by the exchange interaction. Such models, however, do not take into account the strong correlations displayed in a wi...
In dieser Arbeit wurde das Adsorptionsverhalten verschiedener Substanzen aus der Gas- oder Flüssigphase an Modellmembranen untersucht. Lipidmembranen spielen in lebenden Organismen eine wesentliche Rolle. In Form von Doppelschichten organisieren sie die Abgrenzung der Zelle und der intrazellulären Kompartimente. In der Lunge reguliert eine komplexe Lipid-Protein Monolage, das sogenannte pulmonale Surfactant, den störungsfreien Gasaustausch. Heutzutage ist die menschliche Lunge vielen potenzie...
In this work, we are searching for supersymmetric extensions of the Standard Model (SM) of particle physics which are asymptotically safe. Such models are well-defined at all energy scales and provide hints for the scale at which supersymmetry gets broken. The combination of supersymmetry and asymptotic safety hereby turns out to strongly restrict the space of possible models. Within extensions of the minimal supersymmetric SM (MSSM), we perturbatively find candidates which all have a specifi...
The successful implementation of nanoscale materials in next generation optoelectronic devices crucially depends on our ability to functionalize and design low dimensional materials according to the desired field of application. Recently, organic adsorbates have revealed an enormous potential to alter the occupied surface band structure of tunable materials by the formation of tailored molecule-surface bonds. Here, we extend this concept of adsorption-induced surface band structure engineerin...
Organic photovoltaic devices operate by absorbing light and generating current. These two processes are governed by the optical and transport properties of the organic semiconductor. Despite their common microscopic origin—the electronic structure—disclosing their dynamical interplay is far from trivial. Here we address this issue by time-resolved photoemission to directly investigate the correlation between the optical and transport response in organic materials. We reveal that optical gener...
The discovery and realization of graphene as an ideal two-dimensional (2D) material has triggered extensive efforts to create similar 2D materials with exciting spin-dependent properties. Here, we report on a novel Sn 2D superstructure on Au(111) that shows similarities and differences to the expected electronic features of ideal stanene. Using spin- and angle-resolved photoemission spectroscopy, we find that a particular Sn/Au superstructure reveals a linearly dispersing band centered at the ...
The quantification of the electronic transport energy gap of a molecular semiconductor is essential for pursuing any challenge in molecular optoelectronics. However, this remains largely elusive because of the difficulties in its determination by conventional spectroscopic methods. This communication presents an in-device molecular spectroscopy (i-MOS) technique, which permits measuring this gap seamlessly, in real device operative conditions, at room temperature and without any previous know...
Marcus’s theory of electron transfer, initially formulated six decades ago for redox reactionsin solution, is now of great importance for very diverse scientific communities. The molecularscale tunability of electronic properties renders organic semiconductor materials in principlean ideal platform to test this theory. However, the demonstration of charge transfer indifferent Marcus regions requires a precise control over the driving force acting on the chargecarriers. Here, we make use of a ...
Colloidal particles suspended in liquid crystals can exhibit various effective anisotropic interactions that can be tuned and utilized in self-assembly processes. We simulate a two-dimensional system of hard disks suspended in a solution of dense hard needles as a model system for colloids suspended in a nematic lyotropic liquid crystal. The novel event-chain Monte Carlo technique enables us to directly measure colloidal interactions in a microscopic simulation with explicit liquid crystal pa...
We investigate the nonlinear optical response of a thin film of ion-implanted VO2 nanocrystals with open aperture z-scans involving femtosecond near-infrared pulses. Beyond the established nonlinearity related to the insulator-metal phase transition of VO2, the metallic state features a pronounced saturable absorption for 100 fs pulses from a modelocked Yb:fiber source at = 1036 nm. In contrast, we find a pronounced reverse saturable absorption for 90 fs pulses in the telecom window at...
The individual monitoring service at the Materialprüfungsamt North Rhine-Westphalia and the TU Dortmund are developing the compact dosemeter system TL-DOS based on thin-layer thermoluminescence detectors as well as an associated glow curve analysis tool. Various dosemeters of the system measure different dose quantities and types of radiation. This thesis focuses on the TL-DOS neutron dosemeter to measure the whole body dose. The system is optimized in terms of LiF:Mg,Ti detectors, an albedo...
Modern computer processors are nowadays approaching limits due to their quantum limitations. The basic principle of modern electronics is measuring a small electrical charge of electrons passing through electronic circuits. An alternative approach based on novel materials could be the solution, which instead relies on the fundamental quantum- mechanical property – spin. The fundamental requirements that apply to a device based on quantum spin qubits include the ability to scale a quantum syst...
High energy gamma-ray astronomy probes the most extreme phenomena in our universe: super novae and their remnants as well as supermassive black holes at the center of far away galaxies. The First G-APD Cherenkov Telescope (FACT) is a small, prototype Imaging Air Cherenkov Telescope (IACT) operating since 2011 at the Roque de los Muchachos, La Palma, Spain. It specializes in continuously monitoring the brightest known sources of gamma rays. In this thesis, I present a new, open analysis c...
Quantum computers have the potential to speed up certain problems that are hard for classical computers. Hybrid systems, such as the nitrogen vacancy (NV) center in diamond, are among the most promising systems to implement quantum computing, provided the control of the different types of qubits can be efficiently implemented. In the case of the NV center, the anisotropic hyperfine interaction allows one to control the nuclear spins indirectly, through gate operations targeting the elect...
The combination of magnetic resonance with laser spectroscopy provides some interesting options for increasing the sensitivity and information content of magnetic resonance. This review covers the basic physics behind the relevant processes, such as angular momentum conservation during absorption and emission. This can be used to enhance the polarization of the spin system by orders of magnitude compared to thermal polarisation as well as for detection with sensitivities down to the level of ...
In the mitotic spindle microtubules attach to kinetochores via catch bonds during metaphase, and microtubule depolymerization forces give rise to stochastic chromosome oscillations. We investigate the cooperative stochastic microtubule dynamics in spindle models consisting of ensembles of parallel microtubules, which attach to a kinetochore via elastic linkers. We include the dynamic instability of microtubules and forces on microtubules and kinetochores from elastic linkers. A one-sided mode...